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dc.contributor.authorElool Dov, N-
dc.contributor.authorSreejith, S-
dc.contributor.authorCohen, D-
dc.contributor.authorBendikov, T-
dc.contributor.authorRechav, K-
dc.contributor.authorLinda, J W S-
dc.contributor.authorLahav, M-
dc.contributor.authorVan Der Boom, M E-
dc.identifier.citationJournal of the American Chemical Society, 139(33):11471-11481en_US
dc.description.abstractIn this study, we demonstrate a versatile approach for the formation of electrochromic nanoscale assemblies on transparent conductive oxides on both rigid and flexible substrates. Our method is based on the application of alternating spin-coated layers of well-defined metal polypyridyl complexes and a palladium(II) salt to form electrochemically addressable films with a high chromophore density. By varying the central metal ion of the polypyridyl complexes (Os, Ru, and Fe) and their ligands and by mixing these complexes, coatings with a wide range of colors can be achieved. These coatings cover a large area of RGB color space. The coloration intensities of these nanoscale films can be tuned by the number of deposition steps. The materials have very attractive ON/OFF ratios, electrochemical stabilities, and coloration efficiencies. Reversible color-to-colorless and color-to-color transitions were demonstrated, and the films were further integrated into sandwich cells.en_US
dc.publisherAmerican Chemical Societyen_US
dc.titleElectrochromic Metallo-Organic Nanoscale Films: Fabrication, Color Range, and Devicesen_US
Appears in Collections:2017

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